Thermodynamic description of the Cu-Ni-Pb system

• Authors: Jyrki Miettinen , Vania Gandova , Spas Georgiev , Gueorgui Vassilev
• Languages of publication: EN

Abstracts

EN

Thermodynamic description is presented for the ternary Cu-Ni-Pb system. Optimized parameters of the sub-systems, Cu-Ni, Cu-Pb and Ni-Pb, are taken from earlier assessments and those of the ternary system are optimized in this study by using the experimental phase equilibrium and thermodynamic data. Better agreement is obtained by the present optimization. Calculated results are compared with the original experimental data to demonstrate the successfulness of this assessment. Moreover, a geometric model (general solution model) is used to estimate ternary integral molar Gibbs excess energies of the liquid phase from the bibary systems only. These values, however, disagree with the quantities obtained by thermodynamic optimizations. [...]

Keywords

EN

Cu-Ni-Pb system; Thermodynamic optimization; General solution model; Substitutional solution model

• Publisher: De Gruyter Open
• Journal: Open Chemistry
• Year: 2011
• Volume: 9
• Issue: 4
• Pages: 743-749

Dates

published

1 - 8 - 2011

online

4 - 6 - 2011

Contributors

author

Jyrki Miettinen

• Laboratory of Metallurgy, Vuorimiehentie 2K, Helsinki University of Technology, Helsinki, FIN-02015, Finland

author

Vania Gandova

• Faculty of Chemistry, University of Plovdiv, 4000, Plovdiv, Bulgaria

author

Spas Georgiev

• Faculty of Chemistry, University of Plovdiv, 4000, Plovdiv, Bulgaria

author

Gueorgui Vassilev

• Faculty of Chemistry, University of Plovdiv, 4000, Plovdiv, Bulgaria

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Identifiers

DOI

10.2478/s11532-011-0052-4