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Activity and stereoselectivity of Ru-based catalyst bearing a fluorinated imidazolinium ligand

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Siano V., D’Auria I., Grisi F., Costabile C., Longo P.
Open Chemistry
|
2011
|
vol. 9
|
issue 4
605-609
EN
Grubbs II generation catalyst (3), bearing a fluorinated imidazolinium ligand, was investigated in cross metathesis (CM), ring closing metathesis (RCM) and ring opening polymerization metathesis (ROMP) for a variety of substrates. Kinetic studies showed reduced stability of the catalyst in methylene chloride following the first 15 minutes of reaction preventing a higher efficiency despite the very high activity. Beneficial solvent effects on the catalyst stability were observed by performing RCM in C6F6. [...]
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