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Soft magnetic composites represent a remarkable kind of materials with wide variety of use. Magnetic properties are dependent on the materials composition and also on the method of preparation. Ni-Fe-Mo alloys (supermalloy) have high complex permeability and low eddy current losses. Soft magnetic NiZnFe₂O₄ ferrites have low coercivity and intermediate saturation magnetization. The Ni_{80}Fe_{14.7}Mo_{4.5}Mn_{0.5}Si_{0.3} (wt%) powder sample was prepared by mechanical alloying of the chemical elements for 24 h. Ni_{0.3}Zn_{0.7}Fe₂O₄ ferrite is commercially available by Sigma Aldrich. Both powders were mixed at selected ratio and uniaxially compacted at 800 MPa. In this paper, we report the experimental observations of the effects of Ni_{0.3}Zn_{0.7}Fe₂O₄ content on the electromagnetic properties of NiFeMoMnSi/Ni_{0.3}Zn_{0.7}Fe₂O₄. The samples contained 5, 10, and 15% of Ni_{0.3}Zn_{0.7}Fe₂O₄ ferrite and were sintered for 30 min at 800°C. An addition of Ni_{0.3}Zn_{0.7}Fe₂O₄ ferrite caused decrease of complex permeability and increase coercivity of the samples. The 5% of Ni_{0.3}Zn_{0.7}Fe₂O₄ sample exhibits the highest value of the real part of complex permeability (48 at 1 kHz). The 10% of Ni_{0.3}Zn_{0.7}Fe₂O₄ sample showed the lowest total magnetic losses.
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