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Palladium(0)-catalyzed amination of allylic natural terpenic functionalized olefins

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Houssame S., Anane H., Firdoussi L., Karim A.
Open Chemistry
|
2008
|
vol. 6
|
issue 3
470-476
EN
The palladium(0) catalyzed amination of allylic acetates and carbonates derivatives from terpenic olefins was carried out under mild conditions. The reaction offers a very good method for the preparation of allylic amines and thus to provide a useful entry to new functionalized terpenic olefin products. The mechanism involving a formation of p-allyl-palladium intermediate complex is in good agreement with the results obtained with the optically active substrates, as well as via an analysis of the observed regio-and stereoselectivity. [...]
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