We have discussed new optical potentialities in acentric Gd_{2}(MoO_{4})_{3} and LaBGeO_{5} laser crystal-hosts having simultaneously relatively high χ^{(2)} and χ^{(3)} nonlinear susceptibilities. In particular, we show experimental results on efficient multiple Stokes and anti-Stokes stimulated Raman scattering and Raman induced four-wave mixing, as well as second harmonic generation with Cerenkov-type phase matching.
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