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Terrylene in a 2,3-Dichloronaphthalene Crystal. New System for Optical Single-Molecule Investigations

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Białkowska M., Chaładaj W., Makarewicz A., Kozankiewicz B.
Acta Physica Polonica A
|
2015
|
vol. 128
|
issue 3
RK.128.3.1-1-RK.128.3.1-4
EN
Results of optical studies of a new single-molecule system, terrylene molecules in a 2,3-dichloronaphthalene crystal, are presented for the first time. Analysis of the second-order fluorescence intensity correlation function shows that the external heavy-atom effect (due to the chlorine atoms) contributes to the increase of the intersystem crossing rate constant for the S₁ → T₁ transition, by one order of magnitude, whereas the rate constant for the T₁ → S₀ transition is only weakly influenced.
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