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1
Content available remote

Dielectric response of metallic crystal made up of highly polarisable molecules: the semi-classical approach

100%
Bonačić Lošić Ž., Županović P.
Open Physics
|
2009
|
vol. 7
|
issue 4
721-730
EN
The dielectric response is considered within models of a one-band metal, a two-band insulator and a two-band metal using the semi-classical approximation. Corresponding dielectric functions are found. The dielectric function of two-band metal is found to be the interpolation between the Sellmeyer and Lorenz-Lorentz expressions, respectively. The frequencies of the collective modes are identified as the zeroes of the dielectric functions. The correspondence between the semi-classical approach used in this paper and the many-body calculation within the random-phase approximation is established.
2
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Microwave X-Band Resonances in Doped Cd₂Nb₂O₇ Monocrystals

84%
Waplak S., Ostrowski A., Wencka M., Bednarski W.
Acta Physica Polonica A
|
2017
|
vol. 132
|
issue 1
7-11
EN
Cadmium pyroniobiate (CNO) is the ferroic material with unusual diffuse phase diagram which includes both relaxor and nanocluster domains. We present the data for CNO crystals with several admixtures of paramagnetic ions studied on X and S microwave bands at zero-external magnetic field and classical EPR conditions. Our results lead to an assertion of a ferroelectric resonance effect due to "electronic ferroelectricity". The data fit well to the Falicov-Kimball theoretical model applicable to strongly-correlated-electron or mixed-valence systems.
3
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Structural and electrical properties of KCa2Nb5O15 ceramics

84%
Behera B., Nayak P., Choudhary R.
Open Physics
|
2008
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vol. 6
|
issue 2
289-295
EN
A polycrystalline sample of KCa2Nb5O15 with tungsten bronze structure was prepared by a mixed oxide method at high temperature. A preliminary structural analysis of the compound showed an orthorhombic crystal structure at room temperature. Surface morphology of the compound shows a uniform grain distribution throughout the surface of the sample. Studies of temperature variation on dielectric response at various frequencies show that the compound has a transition temperature well above the room temperature (i.e., 105°C), which was confirmed by the polarization measurement. Electrical properties of the material have been studied using a complex impedance spectroscopy (CIS) technique in a wide temperature (31–500°C) and frequency (102–106 Hz) range that showed only bulk contribution and non-Debye type relaxation processes in the material. The activation energy of the compound (calculated from both the loss and modulus spectrum) is same, and hence the relaxation process may be attributed to the same type of charge carriers. A possible ‘hopping’ mechanism for electrical transport processes in the system is evident from the modulus analysis. A plot of dc conductivity (bulk) with temperature variation demonstrates that the compound exhibits Arrhenius type of electrical conductivity.
4
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Structural, dielectric, electrical and piezoelectric properties of Ba4SrRTi3V7O30 (R=Sm, Dy) ceramics

84%
Sahoo P., Panigrahi A., Patri S., Choudhary R.
Open Physics
|
2008
|
vol. 6
|
issue 4
843-848
EN
Polycrystalline samples of Ba4SrRTi3V7O30 (R=Sm and Dy), members of the tungsten-bronze family, were prepared using a high-temperature, solid-state reaction technique and studied their electrical properties (using complex impedance spectroscopy) in a wide range of temperature (31–500°C) and frequency (1 kHz-1 MHz). Preliminary structural (XRD) analyses of these compounds show the formation of single-phase, orthorhombic structures at room temperature. The scanning electron micrographs (SEM) provided information on the quality of the samples and uniform distribution of grains over the entire surface of the samples. Detailed studies of the dielectric properties suggest that they have undergone ferroelectric-paraelectric phase transition well above the room temperatures (i.e., 432 and 355°C for R= Sm and Dy, respectively, at frequency 100 kHz). Measurements of electrical conductivity (ac and dc) as a function of temperature suggest that the compounds have semiconducting properties much above the room temperature, with negative temperature coefficient of resistance (NTCR) behavior. The existence of ferroelectricity in these compounds was confirmed from a polarization study.
5
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Phase transition in Bi8Fe6Ti3O27 multiferroic ceramics

84%
Patri S., Choudhary R.
Open Physics
|
2008
|
vol. 6
|
issue 3
450-453
EN
The polycrystalline Bi8Fe6Ti3O27 compound was prepared by a high-temperature solid-state reaction technique. Preliminary structural analysis by X-ray diffraction (XRD) confirms the formation of a single-phase compound in an orthorhombic crystal system at room temperature. The elemental content of the compound was analyzed by EDAX microanalysis. Microstructural analysis by scanning electron microscopy (SEM) shows that the compound has well defined grains, which are distributed uniformly throughout the surface of the pellet sample. Detailed studies of temperature-dependent dielectric response at various frequencies show dielectric anomalies at 380, 389 and 403°C for 10 kHz, 100 kHz, and 1 MHz respectively. The hysteresis loop observed by applying an electric field of 12 kV/cm on the poled sample with smaller remanent polarization supports the existence of ferroelectricity in this material. The value of d33 of the compound was found to be 19 pC/N.
6
Content available remote

Left-handed chiral metamaterials

84%
Sabah C.
Open Physics
|
2008
|
vol. 6
|
issue 4
872-878
EN
In this work, the concept of left-handed chiral metamaterials is analyzed by emphasizing their optical ability on the rotation of the plane of polarization of a wave. The possibilities of a negative phase velocity, negative and positive propagation constants, and basic electromagnetic properties of this novel medium are also presented. After the characterization of left-handed chiral metamaterial, we provide a reflection and transmission study for two planar boundaries of nonchiral-left-handed chiral metamaterial for normal angles of incidence. Some numerical results are also provided to validate the formulation found in the analysis and to show the role of the chirality in the propagation constants, phase velocities, reflection and transmission.
7
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Band structure and optical properties of antimony-sulfobromide: density functional calculation

84%
Akkus H., Mamedov A., Kazempour A., Akbarzadeh H.
Open Physics
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2008
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vol. 6
|
issue 1
64-75
EN
The electronic structure, linear, and non-linear optical properties of ferroelectric-semiconductor SbSBr are investigated in the non-polar (paraelectric) and polar (ferroelectric) phase, using the density functional methods in the generalized gradient approximation. The electronic band structure obtained shows that SbSBr has an indirect forbidden gap of 2.16 and 2.21 eV in the paraelectric and ferroelectric phase, respectively. The linear photon-energy dependent dielectric functions and some optical functions, such as absorption and extinction coefficients, refractive index, energy-loss function, reflectivity, and optical conductivity in both phases and photon-energy dependent second-order susceptibilities in the ferroelectric phase are calculated. Moreover, some important optical parameters, such as the effective number of valence electrons and the effective optical dielectric constant, are calculated in both phases.
8
Content available remote

Dielectric properties of Ba3Sr2DyTi3V7O30 ceramics

84%
Sahoo P., Panigrahi A., Patri S., Choudhary R.
Open Physics
|
2010
|
vol. 8
|
issue 4
639-642
EN
A polycrystalline sample, Ba3Sr2DyTi3V7O30, with tungsten bronze structure was prepared by a mixed-oxide method at high temperature (950°C). Preliminary structural analysis of the compound showed an orthorhombic crystal structure at room temperature. Surface morphology of the compound was studied by scanning electron microscopy. The dielectric anomaly at 321°C may be attributed to the ferro-paraelectric phase transitions. This was also confirmed from the appearance of a hysteresis loop. The nature of variation of the ac conductivity and value of activation energy at different temperature regions, suggest that the conduction process is of mixed-type (i.e., ionic-polaronic and space charge generated from the oxygen ion vacancies).
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