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A Spectroscopic Study on the Nonlinear Optical Susceptibilities of Organic Molecules

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Foerier S., Valev V., Koeckelberghs G., Kolmychek I., Aksipetrov O., Verbiest T.
Acta Physica Polonica A
|
2007
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vol. 112
|
issue 5
927-934
EN
We report on the investigation of the spectral dependence of nonlinear optical susceptibilities, that describe second harmonic generation - circular dichroism, the nonlinear optical analogue of circular dichroism. The design and implementation of a state of the art experimental setup, used for the characterization of a series of organic molecules in the near-infrared range, will be discussed. We emphasize on the main characteristics like wavelength control, polarization and data-acquisition to present the setup. Some preliminary results show its strength to detect chirality at the molecular and supramolecular level.
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