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Positronium Formation in Nanostructured Metals

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Čížek J., Melikhova O., Hruška P., Vlček M., Anwand W., Liedke M., Novotný M., Bulíř J.
Acta Physica Polonica A
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2017
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vol. 132
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issue 5
1579-1584
EN
Positronium formation in Au films was studied using a magnetically guided continuous slow positron beam with variable energy. Black Au film with porous morphology was compared with conventional smooth Au film. In the smooth Au film positronium is formed on the film surface only. The black Au film exhibits porous sub-surface region containing micro-cavities interconnected with surface. Positronium is formed on inner surfaces of micro-cavities in the sub-surface region and travels through interconnected cavities towards the surface. 3-γ annihilation of ortho-positronium leaves a clear signature in two-dimensional coincidence Doppler broadening spectra. Measures of 3-γ annihilation contribution calculated from single γ-ray and coincidence Doppler broadening spectra were calculated and compared.
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Positronium Probing of Pores in Zirconia Nanopowders

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Prochazka I., Cizek J., Lukac F., Melikhova O., Hruska P., Anwand W., Liedke M., Konstantinova T., Danilenko I.
Acta Physica Polonica A
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2017
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vol. 132
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issue 5
1564-1567
EN
In the present paper, conventional positron lifetime measurements on selected zirconia-based nanopowders are reported. The nanopowders were doped with various metal cations (Y³⁺, Eu³⁺, Gd³⁺, Lu³⁺ and Mg²⁺). Lifetime experiments were conducted in air and supplemented with mass density measurements. In a range of lifetimes, from a few ns to ≈70 ns, up to two individual lifetime components could be identified. Such observations confirmed positronium (Ps) formation with subsequent ortho-Ps pick-off annihilation as well as the occurrence of pores of different size. Pore sizes were estimated using a shape-free model of the correlation between pore size and ortho-Ps lifetime. The origins of pores are discussed on the basis of the ortho-Ps data in combination with the results of mass density measurements.
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