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Femtosecond X-ray Absorption Spectroscopy οf a Light-Driven Spin-Crossover Process

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Milne C., Pham V., Gawelda W., Nahhas A., van der Veen R., Johnson S., Beaud P., Ingold G., Borca C., Grolimund D., Abela R., Chergui M., Bressler C.

issue 2

391-393

Understanding the initial steps during ultrafast molecular reactions involving large spin state changes is a vital goal in structural dynamics research. These involve knowledge of the geometric structure of the system. Ultrafast X-ray absorption spectroscopy with 50-100 picosecond time resolution establishes the geometric structure of the short-lived (τ = 0.6 ns) high spin state. Here we focus on time-resolved X-ray absorption studies with 160-200 fs temporal resolution to monitor the structural evolution in this spin-conversion process.

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1 Acta Physica Polonica A

1 2010

1 Abela R.

1 Beaud P.

1 Borca C.

1 Bressler C.

1 Chergui M.

1 Gawelda W.

1 Grolimund D.

1 Ingold G.

1 Johnson S.

1 Milne C.

1 Nahhas A.

1 Pham V.

1 van der Veen R.

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Femtosecond X-ray Absorption Spectroscopy οf a Light-Driven Spin-Crossover Process