The values of electronic polarizabilities of La³⁺, Ga³⁺, Si⁴⁺, O²¯ ions are specified using new experimental data about optical activity of La₃Ga₅SiO₁₄ crystals. A calculation technique based on the dipole electron shifting model is applied to estimate linear electrooptic coefficients for the La₃Ga₅SiO₁₄. Wavelength dependences of the both linear electro-optic tensor components r₁₁ and r₄₁ are calculated.
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