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[Ni(en)(H_2O)_4][SO_4]·2H_2O - an S = 1 Molecular Magnet with Easy-Plane Anisotropy

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Tarasenko R., Orendáčová A., Tibenská K., Potočňák I., Kajňaková M., Vlček A., Orendáč M., Feher A.

Acta Physica Polonica A

2008

vol. 113

issue 1

481-484

Structural analysis of [Ni(en)(H_2O)_4][SO_4]·2H_2O was performed and it suggests that the crystal field should play a dominant role in the magnetic properties of the system. This conjecture coincides well with the specific heat and susceptibility behaviour. The analysis confirmed that the compound can be treated as a spin 1 single molecule magnet with nonmagnetic ground state introduced by easy-plane single-ion anisotropy D/k_B≈11 K and neglecting in-plane anisotropy E/D <0.1.

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1 Acta Physica Polonica A

1 2008

1 Feher A.

1 Kajňaková M.

1 Orendáč M.

1 Orendáčová A.

1 Potočňák I.

1 Tarasenko R.

1 Tibenská K.

1 Vlček A.

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[Ni(en)(H_2O)_4][SO_4]·2H_2O - an S = 1 Molecular Magnet with Easy-Plane Anisotropy