Low Temperature Crystal Structure Behaviour of Complex Yttrium Aluminium Oxides YAlO_3 and Y_3Al_5O_{12}

• Authors: A. Senyshyn , L. Vasylechko
• Languages of publication: EN

Abstracts

EN

Crystal structures of two yttrium aluminium oxides, namely YAlO_3 and Y_3Al_5O_{12}, were investigated in the temperature range 3.4-300 K by high-resolution neutron powder diffraction. Neither traces of phase transformations nor discontinuous changes of physical properties were observed. Thermal expansion of yttrium aluminium oxides was evaluated in terms of 1st order Grüneisen approximation, where the Debye temperatures and the Grüneisen parameters have been estimated for both compositions. Anomalies in the thermal expansion of yttrium aluminium perovskite have been observed and modelled using the Einstein oscillator with negative Grüneisen parameter. Extended bond length analysis revealed significant thermally-driven modifications of the aluminium-oxygen framework.

Keywords

EN

61.66.Fn; 61.05.F-; 65.40.De; 65.60.+a; 63.70.+h

Discipline

• 61.66.Fn: Inorganic compounds
• 63.70.+h: Statistical mechanics of lattice vibrations and displacive phase transitions
• 65.40.De: Thermal expansion; thermomechanical effects
• 65.60.+a: Thermal properties of amorphous solids and glasses: heat capacity, thermal expansion, etc.
• 61.05.F-: Neutron diffraction and scattering

• Publisher: Institute of Physics, Polish Academy of Sciences
• Journal: Acta Physica Polonica A
• Year: 2013
• Volume: 124
• Issue: 2
• Pages: 329-335

Dates

published

2013-08

Contributors

author

A. Senyshyn

• Forschungs-Neutronenequelle Heinz Maier-Leibnitz FRM-II, Technische Universität München, Lichtenbergstrasse 1, D-85748 Garching b. München, Germany

author

L. Vasylechko

• Lviv Polytechnic National University, 12 Bandera Str, 79013 Lviv, Ukraine

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Identifiers

DOI

10.12693/APhysPolA.124.329