PL EN


Preferences help
enabled [disable] Abstract
Number of results
Journal
2009 | 7 | 3 | 542-549
Article title

Hydrolysis kinetics of p-nitrophenylpicolinate catalyzed by schiff base Mn(III) complexes in Gemini 16-2-16 micellar solutiony

Content
Title variants
Languages of publication
EN
Abstracts
EN
Two mono-Schiff base Mn(III) complexes (MnL2Cl, L=L1 and L2) were synthesized and employed as artificial hydrolases in catalyzing the hydrolysis of p-nitrophenylpicolinate (PNPP) in Gemini 16-2-16 micellar solution. The effect of different micelles and their complex structures on the catalytic hydrolysis of PNPP is discussed in detail. The observations showed that MnL 22Cl exhibited higher catalytic activity over MnL 12Cl under a comparable condition, which confirmed that an open active centre is essential for modulating the activities of the two enzyme mimics. Moreover, under the conditions employed, hydrolytic rates of PNPP induced by these Mn(III) complexes were faster in Gemini 16-2-16 micelles than that in the micellar solution of cetyltrimethylammonium bromide (CTAB), a conventional analogue of Gemini 16-2-16. [...]
Publisher

Journal
Year
Volume
7
Issue
3
Pages
542-549
Physical description
Dates
published
1 - 9 - 2009
online
21 - 6 - 2009
Contributors
author
  • Key Laboratory of Green Chemistry & Technology, School of Chemistry and Pharmaceutical Engineering, Sichuan University of Science & Engineering, Sichuan Zigong, 643000, China
author
  • Key Laboratory of Green Chemistry & Technology, School of Chemistry and Pharmaceutical Engineering, Sichuan University of Science & Engineering, Sichuan Zigong, 643000, China, jwdxb@163.com
author
  • Department of Chemistry and Environment Science, Chongqing University of Arts and Science, Chongqing Yongchuan, 402160, China
author
  • College of Chemistry and Chemical Engineering, West China Normal University, Sichuan Nanchong, 637002, China
author
  • Key Laboratory of Green Chemistry & Technology, School of Chemistry and Pharmaceutical Engineering, Sichuan University of Science & Engineering, Sichuan Zigong, 643000, China
References
  • [1] W. Zeng et al., Adv. Synth. Catal. 346, 1385 (2004) http://dx.doi.org/10.1002/adsc.200404094[Crossref]
  • [2] R. Krishnan, S. Vancheesan, J. Mol. Catal. A-Chem. 142, 377 (1999) http://dx.doi.org/10.1016/S1381-1169(98)00346-X[Crossref]
  • [3] T. Tsumaki, Bull. Chem. Soc. Jpn. 13, 252 (1938) http://dx.doi.org/10.1246/bcsj.13.252[Crossref]
  • [4] D. Chen, A.E. Martell, Inorg. Chem. 26, 1026 (1987) http://dx.doi.org/10.1021/ic00254a013[Crossref]
  • [5] W. Zhang, J.L. Loebach, S.R. Wilson, E.N. Jacobsen, J. Am. Chem. Soc. 112, 2801 (1990) http://dx.doi.org/10.1021/ja00163a052[Crossref]
  • [6] E.N. Jacobsen, L. Deng, Tetrahedron 50, 4323 (1994) http://dx.doi.org/10.1016/S0040-4020(01)89369-8[Crossref]
  • [7] T. Yamada, K. Inagawa, T. Nagata, T. Mukaiyama, Chem. Lett. 21, 2231 (1992) http://dx.doi.org/10.1246/cl.1992.2231[Crossref]
  • [8] W.D. Jiang et al., Colloid Surf. A 315, 103 (2008) http://dx.doi.org/10.1016/j.colsurfa.2007.07.018[Crossref]
  • [9] W.D. Jiang et al., J. Chem. Sci. 120, 411 (2008) http://dx.doi.org/10.1007/s12039-008-0065-5[Crossref]
  • [10] W.D. Jiang et al., Prog React. Kinet. Mec. 31, 11 (2006) [Crossref]
  • [11] W.D. Jiang et al., J. Disper. Sci. Tech. 27, 869 (2006) http://dx.doi.org/10.1080/01932690600719297[Crossref]
  • [12] W.D. Jiang et al., J. Disper. Sci. Tech. 27, 879 (2006) http://dx.doi.org/10.1080/01932690600719321[Crossref]
  • [13] J.Z. Li et al., Transit. Met. Chem. 31, 487 (2006) http://dx.doi.org/10.1007/s11243-006-0019-z[Crossref]
  • [14] X.M. Kou et al., J. Mol. Catal. A-Chem. 210, 23 (2004) http://dx.doi.org/10.1016/j.molcata.2003.09.004[Crossref]
  • [15] Z.S. Zhang, X.M. Yu, L.K. Fong, L.D. Margerum, Inorg. Chim. Acta 317, 72 (2001) http://dx.doi.org/10.1016/S0020-1693(01)00424-8[Crossref]
  • [16] M. Scarpellini et al., Inorg. Chem. 42, 8353 (2003) http://dx.doi.org/10.1021/ic026277c[Crossref]
  • [17] T. Itoh et al., Bull. Chem. Soc. Jpn. 69, 1265 (1996) http://dx.doi.org/10.1246/bcsj.69.1265[Crossref]
  • [18] A. Nomura, Y. Sugiura, Inorg. Chem. 43, 1708 (2004) http://dx.doi.org/10.1021/ic034931y[Crossref]
  • [19] J. Fendler, Membrane Mimetic Chemistry (Wiley, New York, 1982) 339
  • [20] C.A. Bunton, G. Savelli, Adv. Phys. Org. Chem. 22, 213 (1986) http://dx.doi.org/10.1016/S0065-3160(08)60169-0[Crossref]
  • [21] Ch. Rav-Acha, I. Ringel, S. Sarel, J. Katzhendler, Tetrahedron 44, 5879 (1988) http://dx.doi.org/10.1016/S0040-4020(01)81445-9[Crossref]
  • [22] F. Valérie, B. Alain, L. Pierre, J. Mol. Catal. 85, 45 (1993) http://dx.doi.org/10.1016/0304-5102(93)87122-O[Crossref]
  • [23] P. Scrimin, P. Tecilla, U. Tonellato, C.A. Bunton, Colloids Surf. A 144, 71 (1998) http://dx.doi.org/10.1016/S0927-7757(98)00652-9[Crossref]
  • [24] F. Mancin, P. Tecilla, U. Tonellato, Langmuir 16, 227 (2000) http://dx.doi.org/10.1021/la9909594[Crossref]
  • [25] P. Scrimin, P. Tecilla, U. Tonellato, J. Org. Chem. 56, 161 (1991) http://dx.doi.org/10.1021/jo00001a033[Crossref]
  • [26] F. Hampl, F. Liska, F. Mancin, P. Tecilla, U. Tonellato, Langmuir 15, 405 (1999) http://dx.doi.org/10.1021/la980861+[Crossref]
  • [27] R. Fornasier, P. Scrimin, P. Tecilla, U. Tonellato, J. Am. Chem. Soc. 111, 224 (1989) http://dx.doi.org/10.1021/ja00183a034[Crossref]
  • [28] B.Y. Jiang et al., Colloids Surf. A 235, 145 (2004) http://dx.doi.org/10.1016/j.colsurfa.2003.10.019[Crossref]
  • [29] S. Tascioglu, Tetrahedron 52, 11113 (1996) http://dx.doi.org/10.1016/0040-4020(96)00669-2[Crossref]
  • [30] S. Bhattacharya, V.P. Kumar, J. Org. Chem. 69, 559 (2004) http://dx.doi.org/10.1021/jo034745+[Crossref]
  • [31] S. Bhattacharya, V.P. Kumar, Langmuir 21, 71 (2005) http://dx.doi.org/10.1021/la048858f[Crossref]
  • [32] L.G. Qiu, A.J. Xie, Y.H. Shen, J. Mol. Catal. A-Chem. 244, 58 (2006) http://dx.doi.org/10.1016/j.molcata.2005.08.044[Crossref]
  • [33] L.G. Qiu, X. Jiang, L.N. Gu, G. Hu, J. Mol. Catal. A-Chem. 277, 15 (2007) http://dx.doi.org/10.1016/j.molcata.2007.07.028[Crossref]
  • [34] W.D. Jiang et al., J. Colloid Interf. Sci. 311, 530 (2007) http://dx.doi.org/10.1016/j.jcis.2007.02.056[Crossref]
  • [35] H. Chaimovich, I.M. Cuccovia, Quantitative analysis of reagent distribution and reaction rates in vesicles. Progress in Colloid and Polymer Science (Springer Press, Berlin, 1997) 67 [Crossref]
  • [36] D.S. Sigman, C.T. Gutsche, J. Am. Chem. Soc. 94, 1724 (1972) http://dx.doi.org/10.1021/ja00760a051[Crossref]
  • [37] R. Zana, M. Benrraou, R. Rueff, Langmuir 7, 1072 (1991) http://dx.doi.org/10.1021/la00054a008[Crossref]
  • [38] F.M. Menger, J.S. Keiper, Angew. Chem. Int. Ed. 39, 1906 (2000) http://dx.doi.org/10.1002/1521-3773(20000602)39:11<1906::AID-ANIE1906>3.0.CO;2-Q[Crossref]
  • [39] J.G.J. Weijnen, A. Koudijs, G.A. Schellekens, J.F.J. Engbersen, J. Chem. Soc. Perkin Trans. II 829 (1992) [Crossref]
  • [40] T.H. Fife, T.J. Przystas, J. Am. Chem. Soc. 104, 2251 (1982) http://dx.doi.org/10.1021/ja00372a024[Crossref]
  • [41] T.H. Fife, T.J. Przystas, J. Am. Chem. Soc. 107, 1041 (1985) http://dx.doi.org/10.1021/ja00290a048[Crossref]
  • [42] H. Sigel, Angew. Chem. Int. Ed. 14, 394 (1975) http://dx.doi.org/10.1002/anie.197503941[Crossref]
  • [43] T.S. Choi, Y. Shimizu, H. Shirai, K. Hamada, Dyes Pigm. 45, 145 (2000) http://dx.doi.org/10.1016/S0143-7208(00)00015-2[Crossref]
  • [44] F. Alfani et al., Appl. Biochem. Biotechnol. 88, 1 (2000) http://dx.doi.org/10.1385/ABAB:88:1-3:001[Crossref]
  • [45] E. Abuin, E. Lissi, R. Duarte, Langmuir 19, 5374 (2003) http://dx.doi.org/10.1021/la030050s[Crossref]
  • [46] T. Lu, J. Huang, Z. Li, S. Jia, H. Fu, J. Phys. Chem. B. 112, 2909 (2008) http://dx.doi.org/10.1021/jp0766205[Crossref]
  • [47] T. Lu, J. Huang, D. Liang, Langmuir 24, 1740 (2008) http://dx.doi.org/10.1021/la702832v[Crossref]
  • [48] L. Zhou, X. Jiang, Y. Li, Z. Chen, X. Hu, Langmuir 23, 11404 (2007) http://dx.doi.org/10.1021/la701154w[Crossref]
  • [49] J. Chlebicki, J. Wegrzynska, K.A. Wilk, J. Colloid Interf. Sci. 323, 372 (2008) http://dx.doi.org/10.1016/j.jcis.2008.04.011[Crossref]
  • [50] J.E. Klijn et al., J. Phys. Chem. B. 110, 21694 (2006) http://dx.doi.org/10.1021/jp064774z[Crossref]
  • [51] X. Wang, J. Wang, Y. Wang, H. Yan, P. Li, R.K. Thomas, Langmuir 20, 53 (2004) http://dx.doi.org/10.1021/la0351008[Crossref]
  • [52] A. Rodríguez et al., J. Colloid Interf. Sci. 313, 542 (2007) http://dx.doi.org/10.1016/j.jcis.2007.04.049[Crossref]
  • [53] D. Landini, F. Rolla, J. Org. Chem. 47, 154 (1982) http://dx.doi.org/10.1021/jo00340a037[Crossref]
  • [54] C.J. O’Connor, R.E. Ramage, A.J. Porter, Adv. Colloid Interf. Sci. 15, 25 (1981) http://dx.doi.org/10.1016/0001-8686(81)80002-4[Crossref]
Document Type
Publication order reference
Identifiers
YADDA identifier
bwmeta1.element.-psjd-doi-10_2478_s11532-009-0043-x
JavaScript is turned off in your web browser. Turn it on to take full advantage of this site, then refresh the page.