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2012 | 1 | 11-21

Article title

Steam reforming of methane over Ni-substituted Sr hexaaluminates

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EN

Abstracts

EN
Ni-substituted Sr-aluminates Sr1-xNixAl11.2+xNi0.8-xO19-δ (x = 0; 0.2; 0.4; 0.8) obtained by a precipitation method and calcined at 1200°C have been characterized by different physicochemical techniques and their catalytic properties have been tested in steam reformation of methane. It has been shown that substitution of Al3+ and/or Sr2+ by Ni2+ in the aluminate structure results in changes of phase composition, specific surface area, and reducibility of samples. It has been established that the samples are not completely reduced in the temperature range of 30-900°C. The Sr1-xNixAl11.2+xNi0.8-xO19-δ (x = 0; 0.2; 0.4) catalysts are active and stable in the steam reforming of methane at 700oC: residual amount of methane is (1.1±1.0) vol.%, while the Sr1-xNixAl11.2+xNi0.8-xO19-δ (x = 0.8) sample is rapidly deactivated by coking.

Publisher

Year

Volume

1

Pages

11-21

Physical description

Dates

received
16 - 4 - 2012
accepted
29 - 5 - 2012
online
9 - 8 - 2012

Contributors

  • Boreskov Institute of Catalysis, Pr. Akademika Lavrentieva 5, 630090, Novosibirsk, Russian Federation
  • Boreskov Institute of Catalysis, Pr. Akademika Lavrentieva 5, 630090, Novosibirsk, Russian Federation
  • Boreskov Institute of Catalysis, Pr. Akademika Lavrentieva 5, 630090, Novosibirsk, Russian Federation
  • Boreskov Institute of Catalysis, Pr. Akademika Lavrentieva 5, 630090, Novosibirsk, Russian Federation
author
  • Boreskov Institute of Catalysis, Pr. Akademika Lavrentieva 5, 630090, Novosibirsk, Russian Federation
  • Boreskov Institute of Catalysis, Pr. Akademika Lavrentieva 5, 630090, Novosibirsk, Russian Federation
  • Boreskov Institute of Catalysis, Pr. Akademika Lavrentieva 5, 630090, Novosibirsk, Russian Federation
  • Boreskov Institute of Catalysis, Pr. Akademika Lavrentieva 5, 630090, Novosibirsk, Russian Federation

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Document Type

Publication order reference

Identifiers

YADDA identifier

bwmeta1.element.-psjd-doi-10_2478_cse-2012-0002
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