Iron-catalyzed hydrogenation and
dehydrogenation reactions with relevance to
reversible hydrogen storage applications

• Authors: Thomas Zell , Robert Langer
• Languages of publication: EN

Abstracts

EN

Today’s energy concerns require the development
of suitable solutions for the storage of energy from renewable
resources. Although the chemical storage of energy using
molecular hydrogen as energy carrier is one of the best
options, this type of energy storage requires the conversion
of hydrogen to liquid organic hydrogen careers (LOHCs)
for practical reasons. This goal is challenging and highly
desirable at the same time. In comparison to dihydrogen,
hydrogen storage in LOHCs offers easier handling and
minimum dangers involved in their production, storage,
and reconversion. To achieve efficient processes based on
LOHCs highly active catalyst systems are required which
ideally are based on cheap and abundant metals such
as iron. This review summarizes recent advances in ironcatalyzed
hydrogenation and dehydrogenation reactions,
with relevance to reversible hydrogen storage in small
molecules. It entails the dehydrogenation reactions of formic
acid and methanol water mixtures, the reverse reaction,
the hydrogenation of CO2, dehydrogenation of alcohols,
and the hydrogenation of different carbonyl compounds as
the formal reverse reaction, as well as hydrogenation and
dehydrogenation reactions of N-heterocyclic compounds
and hydrogen release reactions from amino boranes.

Keywords

EN

Iron; hydrogenation; dehydrogenation; hydrogen storage

• Publisher: De Gruyter Open
• Journal: Recyclable Catalysis
• Year: 2015
• Volume: 2
• Issue: 1

Dates

accepted

12 - 11 - 2015

online

22 - 2 - 2016

received

30 - 3 - 2015

Contributors

author

Thomas Zell

• ADAMA Makhteshim Ltd., PO Box 60 Industrial
  Zone, Beer Sheva, 8410001, Israel

author

Robert Langer

• Philipps-Universität Marburg, Hans-Meerwein-
  Straße, D-35043 Marburg, Germany; and Lehn Institute of Functional
  Materials (LIFM), Sun Yat-Sen University (SYSU), Xingang Road West,
  Guangzhou 510275, P. R. China

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Identifiers

DOI

10.1515/recat-2015-0010